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Extra resources for Canonical Problems in Scattering and Potential Theory. Part I
Both shifts may occur also simultaneously, as the molecules couple to several others within three dimensional aggregates. As amorphous aggregates do not have a defined structure their absorption spectrum does not show any characteristic shift, but is simply broadened. Absorption spectra of isolated monomers within perfect solutions may also be shifted slightly depending on the polarity of the solvent molecules. Thereby the whole spectrum is shifted in contrast to the case of well defined aggregates where the shift is band-specific .
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The finding of two similar bands in the fit (Fig. 6b, magenta) proves the quality of the fitting algorithm and shows that also a not shifted Soret band remains within the aggregates, which is broader than that of the monomeric Soret bands. This broadened not red-shifted Soret band within J-aggregates has also been found in the fit of the absorbance of the separated J-aggregate fraction (deposits on the cuvette walls) (Fig. 6c), where the monomeric Soret band residue (magenta) vanished almost completely.